The gasification experiments of coal chars with CO2 were carried out isothermally, with K, Ca, Ni, and Zn chloride catalysts, adopting a thermal gravimetric analyzer (TGA) from 800 to 1100 °C. The kinetic characteristic of the samples were described using the volumetric model (VM), the grain model (GM), and the random pore model (PRM). The morphology patterns of the samples were tested ...
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In the, Wyoming is well known for its abundance of coal, especially in the Powder River Basin region, which meets about 40% of coal demand. Thus people are highly interested in using Wyoming coal as a potential feedstock for producing liquid fuels.
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CO capture and utilization caused more and more public attention because of its environmental impact. The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO and HO mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification. The experiments ...
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Competition and Inhibition Effects during Coal Char Gasification in the Mixture of H2O and CO2. Rui Zhang, Q. H. Wang, Zhongyang Luo, M. Fang, K. Cen. Chemistry. 2013. The mechanisms of char gasification in the mixture of H2O and CO2 are not clear, and some problems are yet to be solved. The LangmuirHinshelwood (LH) model of char ...
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Most of the coal produced in the PRB supports electric power generation in the United States. Starting in the 1990s, many coalfired power plants switched to subbituminous coal from the PRB—which has relatively low sulfur content—to meet tightening Clean Air Act emission 2003, the Powder River Basin yielded more coal than the Appalachian coal basins in the eastern United States.
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As the largest coal mining region and the main coal supply in the United States, Powder River Basin (PRB) coal has a tight connection with this country's power industry and requires special attention in coal gasification studies. Very little investigation of PRB gasification rates in the presence of both CO 2 and steam have been done. As a ...
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DOI: / Corpus ID: ; Catalytic CO 2 gasification of a Powder River Basin coal article{Zhang2015CatalyticC2, title={Catalytic CO 2 gasification of a Powder River Basin coal}, author={Fan Zhang and Deping Xu and Yonggang Wang and Yan Wang and Gao Ying and T. Popa and Maohong Fan}, journal={Fuel Processing Technology}, year={2015}, volume={130}, pages={107116} }
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Electrochemical catalytic coal gasification experiments with Fuxin (FX) coal under a CO2 atmosphere were conducted to evaluate the effects of power and temperature on coal gasification and char structure evolution during electrochemical catalytic gasification (ECG). When the power was 400 W, with temperature increasing from 800 to 1000 °C, the CO content in the gas products increased by % ...
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As a result, fuels with larger surface area and more catalytic components in ash were preferred for increasing the intrinsic reactivity of CO2 gasification particularly for lowrank coals and biomass, respectively. ... Reaction kinetics of Powder River Basin coal gasification in carbon dioxide using a modified drop tube reactor, Fuel, 140 (2015 ...
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Introduction. Catalytic coal gasification has been studied worldwide for nearly 20 years due to its advantages, such accelerating process rate, improving carbon conversion degree, reducing process temperature, and thus decreasing energy consumption and limiting mechanical problems due to moderate conditions in a gasifier, as well as achieving a desired gas composition (Huang et al., 2015).
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The mechanisms of char gasification in the mixture of H2O and CO2 are not clear, and some problems are yet to be solved. The LangmuirHinshelwood (LH) model of char gasification in the mixture of H2O and CO2 and the inhibition effect between charH2O and charCO2 reactions are two controversial issues among these problems. This paper presented new data to elucidate these two issues ...
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The coalbased integrated gasification combined cycle (IGCC) offers the advantages of higher efficiency in separating CO 2 and other pollutants compared to conventional coalfired power plants. The CO 2 collected in the IGCC can be injected into oceans or deep underground geological formations [4].
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Introduction. Nowadays, coal gasification technology is being widely developed to keep up with the soaring energy demand [1], [2]. Partial replacement of H 2 O by CO 2 to realize the gasification of coal with H 2 O/CO 2 mixtures (cogasification) is an important approach that can allow for green, lowcarbon, and sustainable development [3]. Moreover, low temperature gasification should also be ...
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DOE PAGES ® Journal Article: Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. Full Record; Other Related Research; Authors: Zhang, Fan; Fan, Maohong; Huang, Xin; Argyle, Morris D.; Zhang, Bo; Towler, Brian; Zhang, Yulong
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The total yield of the liquid tars increased from wt% for noncatalytic stepwise degradation to wt% for CaO catalyzed stepwise degradation, with an increase of wt%. ... Characterization of the mechanism of gasification of a powder river basin coal with a composite catalyst for producing desired syngases and liquids. Appl Catal, A ...
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The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent.
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Gasification of biomass with CO 2 and H 2 O mixtures in a catalytic fluidised bed. Fuel 2017, 210, 605610. DOI: / Ying Wang, David A. Bell. Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel 2017, 187, 94102. DOI: /
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The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO 2 and H 2 O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification.
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Popa et al. [13]. studied the catalytic steam gasification of a Powder River Basin coal using Na2CO3, and the results demonstrated that the total amounts of H2, CO, CO2 and CH4 generated during the entire gasification with 5 g of dry ashfree coal were,, and mol, respectively, while correspondingly, those with catalyst were ...
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CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst. Full Record; Other Related Research; Authors: Zhang, Fan; Xu, Deping; Wang, Yonggang; Argyle, Morris D.; Fan, Maohong Publication Date: Fri May 01 00:00:00 EDT 2015 Sponsoring Org.: USDOE
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The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent. Sodium...
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The catalytic mechanism is generally described as the added metal element contacting with gasifying agent (H 2 O and/or CO 2 ) produces hydrogen and/or carbon monoxide and a layer of...
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Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel (2017) R. Zhang et al. The effects of specific surface area and ash on char gasification mechanisms in the mixture of H 2 O ... Hydrogen production from high temperature steam catalytic gasification of biochar. Journal of the Energy Institute, Volume 89 ...
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The catalytic gasification of coal using calcium as the catalyst has several advantages over potassium, such as lower costs and corrosiveness, abundant reserves on earth, and facile accessibility. ... 2015 Reaction kinetics of Powder River Basin coal gasification in carbon dioxide using a modified drop tube reactor. Fuel 140, 616625.
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A kinetic characterization of the CO 2 gasification of chars from Chinese lowrank lignite coal is performed by isothermal thermogravimetry. The isothermal condition is 1,073 K, and the CO 2 concentration range is 1090%. Alkali and alkali earth catalysts were used to promote the gasification reactivity.
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DOI: / Corpus ID: ; Catalytic gasification of a Powder River Basin coal article{Popa2013CatalyticGO, title={Catalytic gasification of a Powder River Basin coal}, author={T. Popa and Maohong Fan and Morris D. Argyle and Rachid B. Slimane and David A. Bell and Brian Towler}, journal={Fuel}, year={2013}, volume={103}, pages={161170}, url={https://api ...
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Semantic Scholar extracted view of "Gasification of a South Australian lowrank coal with carbon dioxide and steam: kinetics and reactivity studies" by D. Ye et al. ... Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. ... This work reports on a kinetic study on the gasification of Brazilian mineral coal with steam ...
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A study was carried out in both inert and CO 2 atmosphere to investigate the interaction mechanism of K 2 CO 3 with graphite and coal char during the catalytic gasification of coal char. The formation of K 2 CO 3 catalytic precursors was identified by using series of different techniques. The results obtained in an inert atmosphere show that the interaction between K 2 CO 3 and carbon readily ...
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Highquality oil and gas from pyrolysis of Powder River Basin coal catalyzed by an environmentallyfriendly, inexpensive composite ironsodium catalysts Article Dec 2017
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CO2 gasification of a subbituminous Wyodak coal from the Powder River Basin (PRB) was conducted in a fixedbed laboratory gasifier at atmospheric pressure with FeCO3 as a catalyst precursor.
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Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in Wyoming.
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